Analysis of Rat Blood Samples for Agent Biomarkers After GB Inhalation Exposure

Abstract

A method was developed for the analysis of a GB nerve agent biomarker in blood that is very sensitive, selective, and applicable for archived samples. The biomarker resulting from sample acidification and in the presence of fluoride ion was regenerated GB (rGB) which was found in rat blood after inhalation exposures ranging from miosis to lethal levels. The method utilized a C18 solid-phase extraction (SPE) followed by quantification using a gas chromatograph with either a flame photometric detector (GC-FPD) or a mass spectrometer (GC-MS). Samples were concentrated by injecting the SPE extract on a Tenax -TA sorbent tube along with 100 pg of decadeuterated diethyl ethyl phosphonate as the internal standard followed by thermal desorption GC-FPD analysis and GC-MS confirmation. The method detection limit was 6 pg of agent and the working range was 20-200 pg GB on column. Quality control samples were analyzed and yielded spike recoveries greater than 95%.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2002
Accession Number
ADA436016

Entities

People

  • B. Gaviola
  • C. Crouse
  • D. C. Burnett
  • E. M. Jakubowski
  • H. Dupont Durst
  • J. Anthony
  • J. Manthei
  • L. S. Heykamp
  • R. J. Mioduszewski
  • R. Way
  • S. A. Thomson
  • W. Muse

Organizations

  • Edgewood Chemical Biological Center

Tags

Communities of Interest

  • Biomedical

DTIC Thesaurus Topics

  • Abstracts
  • Biological Markers
  • Blood
  • Cells
  • Chemical Warfare
  • Chemical Warfare Agents
  • Chemical Weapons
  • Detection
  • Detectors
  • Extraction
  • Fluorides
  • Instrumentation
  • Mass Spectrometers
  • Mass Spectrometry
  • Nerve Agents
  • Rodents
  • Standards

Fields of Study

  • Chemistry

Readers

  • Analytical Chemistry
  • Oncology and Biomarker-Based Cancer Detection.