Gas Chromatographic-Mass Spectrometric Determination of British Anti-Lewisite in Plasma

Abstract

British anti-Lewisite (BAL) (2,3-dimercapto-1-propanol) is a potential therapeutic compound when used against the effects of cutaneous sulfur mustard, and a method for its determination in plasma has been developed. BAL and the internal standard (IS) ethane dithiol were isolated from plasma samples through solid-phase extraction and then reacted with 1-pentafluoropropionylimidazole, forming stable pentafluoropropionyl derivates that are sensitive to gas chromatographic-mass spectrometric analysis. Examination of concentration versus peak-area ratios of the BAL and IS derivatives demonstrated the method to be linear over a concentration range of 0.48 to 124 ng(mL in plasma when fit to a weighted (1/y2) least squares regression. Correlation coefficients were 0.9943 to 0.9995 for six runs, and coefficients of variation (CV) were 2.5 to 8.7% over the eight concentrations tested. The intra- and interday accuracy and precision of this method was measured by examining six groups of eight unknown test samples (n = 6).

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Document Details

Document Type
Technical Report
Publication Date
Aug 01, 2004
Accession Number
ADA442484

Entities

People

  • B. R. Capacio
  • C. E. Byers
  • E. D. Clarkson
  • E. R. Holloway
  • G. E. Platoff
  • Joseph P. Smith
  • W. D. Korte

Organizations

  • United States Army Medical Research Institute of Chemical Defense

Tags

DTIC Thesaurus Topics

  • Biomedical Research
  • Blood Proteins
  • Chelate Compounds
  • Chemical Synthesis
  • Chemistry
  • Chlorides
  • Electrons
  • Heavy Metals
  • Liquid Chromatography
  • Mass Spectrometry
  • Organic Chemistry
  • Reaction Time
  • Regression Analysis
  • Rodents
  • Spectrometry

Fields of Study

  • Chemistry

Readers

  • Analytical Chemistry