Growth of Single Crystals and Fabrication of GaN and AlN Wafers

Abstract

GaN thin films were grown on (0001) sapphire substrates at 1050 deg C by controlled evaporation of Ga metal and reaction with NH3. Transport of Ga species from source-to-substrate during this process and the influence of ammonia-liquid Ga reaction on Ga transport were investigated. Experimental results were compared to theoretical predictions to quantify the mechanism of transport in the vapor growth technique. In presence of NH3 Ga transport far exceeded the predicted upper limit for the vapor phase transport. Visual observations confirmed that a significant amount of Ga left the source in a cluster rather than atomic form. Pure N2 was flowed directly above the molten Ga source. This prevented direct contact and reaction between the molten Ga and NH3 and prevented Ga spattering and GaN crust formation on the source surface. It enhanced Ga evaporation rate and enabled control of Ga transport and V/III ratio in the system. The results showed that the process was mass transport limited and the maximum growth rate was controlled by transport of both Ga and reactive ammonia species to the substrate surface.

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 2006
Accession Number
ADA444058

Entities

People

  • Raoul Schlesser
  • Zlatko Sitar

Organizations

  • North Carolina State University

Tags

Communities of Interest

  • Air Platforms
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Boundary Layer
  • Chemical Reactions
  • Compound Semiconductors
  • Crystal Structure
  • Crystals
  • Diffraction
  • Heat Energy
  • Heat Transfer
  • Laser Diodes
  • Materials
  • Materials Science
  • Mechanical Properties
  • Optical Properties
  • Phase Transformations
  • Semiconductors
  • Silicon Carbide
  • Thermodynamics

Fields of Study

  • Materials science

Readers

  • Aviation Safety and Air Traffic Management
  • Combustion science or combustion engineering.
  • Thin Film Deposition Science.