Embedding Luminescent Nanocrystals in Silica Sol-Gel Matrices

Abstract

We have synthesized stable, highly luminescent silica xerogels as well as optically transparent, stable aerogels that were embedded with 2.5 nm and 6 nm CdSe and 6 nm InP quantum dots. By capping the quantum dot with 3-aminopropyltriethoxysilane, a dot is able to condense within the structure of a forming silica gel. This network keeps the quantum dot in place during the solvent exchange procedure necessary to form low-density silica aerogels using supercritical drying procedures. The resulting aerogel networks show a high surface area of 789.7 m2/g and xerogels show a surface area of 448 m2/g, with a pore size of 3.16 nm. Materials created are stable under atmospheric conditions and up to temperatures of 150 C.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2006
Accession Number
ADA445260

Entities

People

  • Lindsey M. Sorensen

Organizations

  • Florida State University

Tags

Communities of Interest

  • Advanced Electronics
  • Biomedical
  • Sensors

DTIC Thesaurus Topics

  • Alcohols
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Climate Change
  • Detection
  • Detectors
  • Liquid Chromatography
  • Materials
  • Materials Laboratories
  • Materials Processing
  • Materials Science
  • Nanocrystals
  • Nanomaterials
  • Optical Properties
  • Optics
  • Quantum Dots

Readers

  • Materials Science and Engineering.
  • Nanocomposite Materials Science
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Quantum Computing