Direct Observation of the Evolution of Both the HOMO and LUMO Energy Levels of a Silole Derivative at a Magnesium/Silole Interface

Abstract

The electronic structure of the interface formed by Mg deposition onto 2,5-bis(6 -(2 ,2 -bipyridyl))-1,1-dimethyl-3,4- diphenyl silacyclopentadiene (PyPySPyPy) was investigated using ultraviolet, inverse, and X-ray photoemission spectroscopies. PyPySPyPy is of interest for use as an electron injection/transport layer in high efficiency organic lightemitting diodes. Upon deposition of Mg onto PyPySPyPy there is a shift of the occupied energy level structure to higher binding energy, away from the Fermi level, and appearance of two energy levels within the energy gap of PyPySPyPy. The lowest unoccupied molecular orbital is also shifted to higher binding energy.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2004
Accession Number
ADA447720

Entities

People

  • A. J. Maekinen
  • Masaki Uchida
  • N. J. Watkins
  • Yifeng Gao
  • Z. H. Kafafi

Organizations

  • United States Naval Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Charge Carriers
  • Charge Transfer
  • Electron Energy
  • Electrons
  • Energy Levels
  • Fermi Levels
  • Kinetic Energy
  • Materials
  • Measurement
  • Optoelectronic Devices
  • Organic Light Emitting Diodes
  • Photoelectric Emission
  • Radiation
  • Spectra
  • Spectroscopy
  • Work Functions
  • X Rays

Readers

  • Quantum Chemistry
  • Solar Photovoltaics and Thermoelectric Devices.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene
  • Space