Monitoring Sulfur Mustard Exposure by the GC-MS Analysis of Thiodiglycol Cleaved from Blood Proteins

Abstract

A GC-MS assay of thiodiglycol (TDG) released from blood protein adducts of sulfur mustard (SM) was developed. Exposure of pig blood to SM (24 nM to 400 nM) resulted in a SM concentration-dependent increase in plasma TDG levels from 2.0 pg/mg protein to 38 pg/mg protein. TDG levels in blood samples drawn from monkeys (Chlorocebus aethiops) after a 1.0 mg/kg intravenous SM injection decreased from 220 pg/mg to 10 pg/mg protein during 45 days. TDG levels in plasma samples from pigs after a 2.4 mL (0.4 ml/site, 6 sites) neat SM percutaneous exposure decreased from 60 pg/mg protein to 4 pg/mg protein during 21 days. This assay was precise, reproducible, and relatively simple with the potential to become a routine test for SM exposure.

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Document Details

Document Type
Technical Report
Publication Date
Nov 18, 2003
Accession Number
ADA453650

Entities

People

  • Benedict R. Capacio
  • Dana R. Anderson
  • Joseph P. Smith
  • Michael Delion
  • William D. Korte

Organizations

  • United States Army Medical Research Institute of Chemical Defense

Tags

Communities of Interest

  • Biomedical

DTIC Thesaurus Topics

  • Abstracts
  • Aspartic Acid
  • Biomedical Research
  • Blood
  • Blood Cells
  • Blood Proteins
  • Carboxylic Acids
  • Cells
  • Chemical Warfare
  • Chemical Warfare Agents
  • Detection
  • Glutamic Acid
  • Mass Spectrometry
  • Molecules
  • Monitoring
  • Proteins
  • Sulfur

Fields of Study

  • Biology

Readers

  • Geochemistry
  • Military Engineering.
  • Toxicology/Environmental Toxicology