Transport Properties of N-Methyloated Nylon-6: Chitosan Blend Membranes

Abstract

A series of N-Methylolated Nylon-6 chitosan blend membranes was evaluated for their potential use as breathable (high water transport) barriers (low chemical agent transport) for military and civilian protective clothing apparel. Nylon-6 was methylolated and subsequently blended with chitosan at different compositions and processing conditions (room temperature, 100 C, and 200 C). Vapor transport rates of water (breathability) and dimethyl methylphosphonate (protection) (a simulant of the nerve agent Sarin) were measured as a function of these blend parameters with the use of a modified ASTM (American Society for Testing Materials) method E-96-95 and were compared to Nafion 117. Water transport rate was found to be between 1,000 and 2,000 g/m2day, depending on specific composition of the membranes and thermal treatment. The effective dimethylmethylphosphonate permeability (a thickness independent value) of the blend membranes was two orders of magnitude lower than Nafion 117. The selectivity of N-Methylolated Nylon-6 chitosan blend was 15.3, seven times higher than Nafion 117. It was shown that these membranes, manufactured when hydrophilic and hydrophobic polymers were conjoined, have resulted in a material that is both breathable and protective. These semi-permeable membranes will be economically attractive for military and civilian applications in the area of personal protection since the polymer components are inexpensive and the membrane fabrication is simple.

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Document Details

Document Type
Technical Report
Publication Date
Sep 01, 2006
Accession Number
ADA455775

Entities

People

  • Eugene G. Napadensky
  • Yossef A Elabd

Organizations

  • United States Army Research Laboratory

Tags

Communities of Interest

  • Human Systems

DTIC Thesaurus Topics

  • Chemical Warfare
  • Chemical Warfare Agents
  • Clothing
  • Fabrication
  • Films
  • Liquid Chromatography
  • Materials
  • Mixtures
  • Nerve Agents
  • Permeability
  • Physical Properties
  • Polymers
  • Protective Clothing
  • Thickness
  • Transport Properties
  • Two Dimensional
  • Water Vapor

Readers

  • Materials Science
  • Nanocomposite Materials Science
  • Polymer Science and Engineering.