Characterization and Optimization of a High Surface Area-Solid Phase Microextraction Sampler for the Collection of Trace Level Volatile Organic Compounds in the Field

Abstract

A prototype rapid, high volume air sampling device based on Solid Phase Microextraction (SPME) has been developed for the collection of trace level volatile organic compounds (VOCs). The High Surface Area-Solid Phase Microextraction (HSASPME) device contains ten times more polymer than traditional SPME fibers and is uniquely designed to optimize compound uptake at higher flow rates. This study evaluated the extraction efficiency at six air sampling flow rates ranging from 0.1 L/min to 10 L/min and compared total compound extraction at the two extreme flow rates. A 10 ppb(v) concentration of 39 volatile organic compounds was used. Carboxen/Poly(dimethylsiloxane) and Poly(dimethylsiloxane) polymer coatings were evaluated using an Agilent 6890N/5973, a resistively heated Low Thermal Mass Gas Chromatograph column and an Entech 7100 Preconcentrator. Larger extraction efficiencies were observed at lower flow rates, but the higher flow rates proved superior in total compound extraction per unit time. Across the range of compounds, the HSASPME device achieved an average 8-fold increase in compound uptake at a flow rate of 10 L/min as compared to 0.1 L/min.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2006
Accession Number
ADA459030

Entities

People

  • Shannon S. Mcdonald

Organizations

  • Uniformed Services University of the Health Sciences

Tags

Communities of Interest

  • Biomedical
  • Energy and Power Technologies
  • Ground and Sea Platforms
  • Space
  • Weapons Technologies

DTIC Thesaurus Topics

  • Air Force
  • Alkenes
  • Boiling Point
  • Chemical Analysis
  • Chemical Synthesis
  • Chemistry
  • Chlorides
  • Detection
  • Environmental Protection
  • Hygiene
  • Mass Spectrometry
  • Medical Personnel
  • Organic Chemistry
  • Organic Compounds
  • Solid Phases
  • Spectrometry
  • Volatile Organic Compounds

Readers

  • Analytical Chemistry
  • Solar Photovoltaics and Thermoelectric Devices.