Large Resonant Third-order Optical Nonlinearity of CdSe Nanocrystal Quantum Dots

Abstract

Resonant third-order nonlinear optical susceptibility and hyperpolarizability of CdSe nanocrystal quantum dots were revealed to be ~2.6 10(exp -20) 2.7 10(exp -19) sq m/V2 and ~2.2 10(exp -40) m5/V2 by using nanosecond degenerate four-wave mixing at 532 nm. The large nonlinearity of the CdSe nanocrystals is attributed to the resonant excitation and multiple nonlinear optical processes.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2006
Accession Number
ADA464160

Entities

People

  • Ashley Jackson
  • Bagher Tabibi
  • Herbert Brown
  • Jaetae Seo
  • Linwood Creekmore
  • Min Namkung
  • Qiguang Yang
  • Russell Battle
  • Seongmin Ma
  • Sungsoo Jung
  • Tifney Skyles
  • William Yu

Organizations

  • Hampton University

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Absorption
  • Absorption Coefficients
  • Absorption Spectra
  • Crystals
  • Ground State
  • Inorganic Carbon Compounds
  • Materials
  • Nanocrystals
  • Nanosecond Time
  • Optical Properties
  • Physics
  • Quantum Dots
  • Refractive Index
  • Semiconductors
  • Wave Mixing

Fields of Study

  • Physics

Readers

  • Mathematics or Statistics
  • Nanoscale Plasmonic Nanotechnology
  • Optical Physics and Photonics.

Technology Areas

  • Quantum Computing