Condensed-Phase Reactions of Energetic Ionic Liquids Under Different Ignition Stimuli

Abstract

The experimental work conducted under this program was designed to provide new insight into condensed-phase reactions leading to ignition of ionic liquids. The objectives of the work were: (1) to identify the initiation and secondary reactions in the condensed phase that lead to ignition and combustion, (2) to understand the effects of the structure of the cation on these reactions, and (3) to determine the effects of the type of ignition stimulus used. Two primary experimental approaches were applied: laser heating coupled with tandem mass spectrometry and rapid thermolysis coupled with FTIR and time-of-flight mass spectrometry. The compounds studied included: l-Ethyl-3-Methyl-Imidazolium Nitrate, 4-Amino-l,2,4-Triazolium Nitrate, i-Methyl, 4-Amino-l,2,4-Triazolium Nitrate, 2-Amino-4,5-Dimethyl Tetrazolium Nitrate and 1-Amino-4,5-Dimethyl Tetrazolium Nitrate.

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Document Details

Document Type
Technical Report
Publication Date
Mar 20, 2007
Accession Number
ADA464980

Entities

People

  • Stefan T. Thynell
  • Thomas A. Litzinger

Organizations

  • Pennsylvania State University

Tags

Communities of Interest

  • C4I

DTIC Thesaurus Topics

  • Barometric Pressure
  • Chemical Synthesis
  • Chemistry
  • Combustion
  • Decomposition
  • Heat Flux
  • Ignition
  • Ionic Liquids
  • Liquids
  • Mass Spectra
  • Mass Spectrometers
  • Materials
  • Measurement
  • Molecular Beams
  • Nitric Acid
  • Spectra
  • Spectroscopy

Fields of Study

  • Chemistry

Readers

  • Combustion science or combustion engineering.
  • Quantum Chemistry
  • Rocket Propulsion.

Technology Areas

  • Directed Energy