Detection of Organophosphorus Compounds by Covalently Immobilized Organophosphorus Hydrolase

Abstract

As a consequence of organophosphorus (OP) toxins posing a threat to human life globally, organophosphorus hydrolase (OPH) has become the enzyme of choice to detoxify such compounds. Organophosphorus hydrolase was covalently immobilized onto a quartz substrate for utilization in paraoxon detection. The substrate was cleaned and modified prior to chemical attachment. Each modification step was monitored by imaging ellipsometry as the thickness increased with each modification step. The chemically attached OPH was labeled with a fluorescent dye (7-isothiocyanato-4-methylcoumarin) for the detection of paraoxon in aqueous solution, ranging from 1 nanomole to 10 micromole. UV-visible spectra were also acquired for the determination of the hydrolysis product of para-oxon, namely p-nitrophenol.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Oct 01, 2006
Accession Number
ADA470902

Entities

People

  • Celeste A. Constantine
  • Jhony Orbulescu
  • Joseph J. Defrank
  • Roger M. Leblanc
  • Saumil S. Shah
  • Vipin K. Rastogi

Organizations

  • University of Miami

Tags

Communities of Interest

  • Counter WMD
  • Sensors

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Abstracts
  • Amines
  • Analytical Chemistry
  • Biochemistry
  • Buffers (Chemistry)
  • Chemical Synthesis
  • Chemistry
  • Chromatography
  • Detection
  • Liquid Chromatography
  • New York
  • Organophosphorus Compounds
  • Pesticides
  • Spectra
  • Spectroscopy

Fields of Study

  • Chemistry

Readers

  • Molecular and Cellular Biochemistry
  • Neurotoxicology
  • Thin Film Deposition Science.