Preliminary Evaluation of the Properties of Dynamically Vulcanised Thermoplastic Rubbers

Abstract

The report presents work on five types of dynamically vulcanized thermoplastic rubber blends made from chlorobutyl and nitrile rubbers and polypropylene, nylon 12, and PPT resins. The project objective was to establish a correlation between blend composition and properties such as microstructure swelling index, tensile strength, elongation at break, hardness, and resistance to penetration/reemission of chemical warfare agents. The method of blend preparation and materials testing was described. Results were reviewed and conclusions were drawn. The results confirm that dynamic vulcanization can produce a variety of rubber plastic blends, many with elastomeric properties. Both rubber and plastic phases seems to be affected during the dynamic vulcanization process. Under exposure to solvents, both vulcanized rubber and rubber/plastic blends underwent a rapid approach to equilibrium swelling. It was found that swelling index values of blends were significantly less that the expected "theoretical" values, based strictly on composition in the blend. This was attributed to a caging effect of the thermoplastic phase on the rubber phase at the higher thermoplastic composition. In blends of rubber and thermoplastic, the minimum elongation at break seems to be reached at phase inversion. With respect to re-emission values for the five blends systems studied, from best to worst, the order is PA/CIIR > PP/CIIR > PA/NBR > PP/NBR > PBT/NBR. Selected results were presented during the IUPAC International Polymer Congress in Paris (July 4-8, 2004). Overheads from the presentation are enclosed with report.

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Document Details

Document Type
Technical Report
Publication Date
Nov 01, 2004
Accession Number
ADA475504

Entities

People

  • J. D. Van Dyke
  • Marek Gnatowski

Organizations

  • Trinity Western University

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Biomedical And Dental Materials
  • Chemical Warfare
  • Chemical Warfare Agents
  • Chemistry
  • Curing
  • Engineering
  • Fatty Acids
  • Hardness
  • Materials
  • Materials Science
  • Materials Testing
  • Mechanical Properties
  • Nitrile Rubber
  • Plastics
  • Resins
  • Tensile Strength
  • Thermoplastic Resins

Fields of Study

  • Materials science

Readers

  • Forest Ecology
  • Mechanical Engineering/Mechanics of Materials.
  • Powder metallurgy of Titanium alloys.