Laser-Induced Breakdown Spectroscopy Infrared Emission From Inorganic and Organic Substances

Abstract

Laser-induced breakdown spectroscopy (LIBS) has been established as a powerful method for identifying trace elemental contaminants by analyzing the atomic spectral emission lines that result subsequent to plasmas generated by laser power. The ultraviolet-visible-near infrared (UV-Vis- NIR) spectral region exploited in conventional LIBS largely elucidates the elemental composition of the laser target by profiling these atomic lines; very limited information on molecular species may be derived. To our best knowledge, there is no reference to LIBS measurements on emission processes outside of the UV-Vis-NIR region. In this pioneer work, attempts were made herein to probe the mid-infrared (MIR) emission from a laserinduced breakdown process between 2 to 5.75 microns. Emission features between 4200 to 4800 nm from oxygenated carbon-containing breakdown fragments and between 2000 to 4000 nm from alkali metal-containing breakdown fragments have been successfully identified. These findings could provide additional spectral information to complement the conventional LIBS analysis and launch a new analytical methodology and sensing method for future contamination avoidance applications.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Nov 01, 2006
Accession Number
ADA481534

Entities

People

  • A. C. Samuels
  • A. P. Snyder
  • C.s. Yang
  • E. Brown
  • S. B. Trivedi
  • U. Hömmerich

Tags

Communities of Interest

  • C4I
  • Energy and Power Technologies
  • Sensors

DTIC Thesaurus Topics

  • Alkali Metals
  • Chemical Synthesis
  • Chemistry
  • Detection
  • Detectors
  • Emission
  • Emission Spectra
  • Emission Spectroscopy
  • Laser Beams
  • Laser Pulses
  • Laser-Induced Breakdown Spectroscopy
  • Lasers
  • Materials
  • Measurement
  • Metals
  • Spectra
  • Spectroscopy

Fields of Study

  • Physics

Readers

  • Optical Physics and Photonics.
  • Organic Chemistry
  • Spectroscopy.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers