Speciation and Geochemistry of Tungsten in Soil

Abstract

In order to limit the dispersive use of lead on small arms firing ranges, 5.56-mm bullets with tungsten-nylon composite material cores have been fired at a number of Army training ranges. Tungsten in bullet residues oxidizes when exposed to the atmosphere, yielding an amorphous tungsten oxide (WO3) coating. This coating rapidly dissolves to yield the tungstate anion (WO4 2-), which can migrate in saturated subsurface and surface water environments. The environmental geochemistry of dissolved tungsten species is complex, and consequently is not well characterized. Tungsten exists in most environmental matrices as the soluble and mobile tungstate anion, which can polymerize with itself and other anions, such as molybdate and phosphate, making determination of tungsten compounds important. Since the geochemical and toxicological properties of these polymer species may vary from monomeric tungstate, determination of tungstate is as critical as determination of total dissolved tungsten concentration.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Nov 01, 2006
Accession Number
ADA481554

Entities

People

  • A. J. Bednar
  • D. B. Ringelberg
  • J. E. Mirecki
  • L. E. Winfield
  • L. S. Inouye
  • S. L. Larson

Organizations

  • Engineer Research and Development Center

Tags

DTIC Thesaurus Topics

  • Chemical Synthesis
  • Chemistry
  • Chromatography
  • Composite Materials
  • Elements
  • Environment
  • Environmental Protection
  • Geochemistry
  • Hydroxides
  • Ion Exchange
  • Liquid Chromatography
  • Mass Spectrometry
  • Metals
  • Spectrometry
  • Tungsten
  • Tungsten Compounds
  • Water

Fields of Study

  • Environmental science

Readers

  • Agricultural Chemistry/Soil Science
  • Materials Science and Engineering.
  • Powder metallurgy of Titanium alloys.