Cathodoluminescence Study of ZnO Wafers Cut from Hydrothermal Crystals

Abstract

ZnO is a wide bandgap semiconductor with very promising expectation for UV optoelectronics. The existence of large crystals should allow homoepitaxial growth of ZnO films for advanced optoelectronic devices. However, the ZnO substrates are not yet mature. Both defect induced by growth and by polishing together with the high reactivity of the surface are problems to their industrial application. Cathodoluminescence (CL) was used to probe the quality of substrates from two different suppliers. The surface damage was studied by varying the penetration depth of the electron beam, allowing to observe significant differences between the two samples within a 0.5-mm-thick surface layer. CL spectra show a complex band (P1) at _3.3 eV composed of two overlapped bands (3.31 and 3.29 eV) related to point defects (PD) and the 1-LO phonon replica of the free exciton (FX-1LO). This band (P1) is shown to be very sensitive to the presence of defects and the surface and thermal treatments. Its intensity compared with the excitonic band intensity is demonstrated to provide criteria about the quality of the substrates.

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Document Details

Document Type
Technical Report
Publication Date
Nov 22, 2008
Accession Number
ADA485655

Entities

People

  • A. Soto Rodríguez
  • Buguo Wang
  • D. Bliss
  • J. Mass
  • José Luis González
  • M. Avella
  • M. Callahan
  • T. Rodriguez

Organizations

  • Air Force Research Laboratory

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Air Force
  • Air Force Research Laboratories
  • Band Gaps
  • Cathodoluminescence
  • Computer Programs
  • Crystal Growth
  • Crystals
  • Energy Bands
  • Excitons
  • Intensity
  • Luminescence
  • Point Defects
  • Polishing
  • Semiconductors
  • Spectra
  • Substrates
  • Wide Bandgap Semiconductors

Fields of Study

  • Materials science

Readers

  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.
  • Thin Film Deposition Science.

Technology Areas

  • Directed Energy
  • Microelectronics
  • Microelectronics - Graphene