Synthesis of New High-Oxygen Carriers and Ditetrazinetetroxide (DTTO)

Abstract

The feasibility of tetranitratoborates and tetranitratoaluminates as high-oxygen carriers for oxidizer balanced green solid and ionic liquid energetic materials was demonstrated. The predicted performances of the ionic liquids represent a marked improvement over liquid energetic materials was demonstrated. The predicted performances of the ionic liquids represent a marked improvement over the presently used hydrazine while avoiding at the same time its high vapor toxicity. Simple, one-pot, one-step syntheses from inexpensive and readily available starting materials have also been developed for these materials. However, the long-term thermal stability of these compound is marginal, and work on an alternate high-oxygen carrying anion has been started. A second area of significant interest was the synthesis of DTTO and iso-DDTO. Theoretical performance calculations were carried out for both using the latest density and heat of formation values, and show that both compounds would provide significantly higher detonation pressures than HMX and CL20. Efforts were started to develop suitable methodology for their syntheses.

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Document Details

Document Type
Technical Report
Publication Date
Dec 24, 2009
Accession Number
ADA513104

Entities

People

  • Cj Jones
  • Karl O. Christe
  • R. Haiges
  • R. I. Wagner

Organizations

  • University of California, Los Angeles

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Anhydrides
  • Chemical Synthesis
  • Chemistry
  • Crystal Lattices
  • Crystal Structure
  • Energetic Materials
  • Explosives
  • Heat Energy
  • Heat Of Formation
  • Ionic Liquids
  • Liquids
  • Materials
  • Materials Science
  • Materials Testing
  • Organic Chemistry
  • Physical Properties
  • Thermal Stability

Fields of Study

  • Chemistry

Readers

  • Combustion science or combustion engineering.
  • Nanocomposite Materials Science
  • Quantum Chemistry