Vibrational Spectroscopic Analysis on the Deformational Behavior of Hybrid Polymers

Abstract

Under this equipment grant, we are to acquire a unique characterization facility needed for determining sub-molecular level changes in the atomic bonding responsible for the enhanced performance of materials reinforced with a new class of nano-structured, hybrid chemicals; polyhedral oligomeric silsesquioxanes (POSS). This facility is vital to the PI's current AFOSR and AFRL-PRSM projects because it will expand the use of POSS in both high temperature polymeric matrix composites and engineering elastomers. This effort is needed for a fundamental advancement of our understanding for the synergistic performance enhancement in the use of nano-structured hybrid chemicals with organic materials. Under this effort, we had purchased 1) an upgrade the existing Fourier transform infrared spectrometer (FT-IR) equipped with a new detector, 2) a micro-Raman spectrometer with 3 different excitation lasers covering from UV to near-IR range, and 3) a custom heated deformation stage. This unique facility with these state-of-the-art spectroscopic techniques will enable a direct measurement on the shifts of vibrational frequencies which are associated with specific molecular segments as the material experiences an externally imposed field, e.g., thermal or mechanical loads. The spectroscopic technique is also a non-destructive method. This information is invaluable as we seek to understand the molecular origins behind the observed performance enhancements in a variety of materials which have been reinforced by functionalized, nano-structured hybrid chemicals such as POSS.

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Document Details

Document Type
Technical Report
Publication Date
Mar 10, 2010
Accession Number
ADA515959

Entities

People

  • Andre Lee

Organizations

  • Michigan State University

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Biomedical And Dental Materials
  • Block Copolymers
  • Chemical Engineering
  • Chemistry
  • Composite Materials
  • Detectors
  • Elastomers
  • Engineering
  • Fiber Reinforced Composites
  • High Temperature
  • Inorganic Materials
  • Materials
  • Materials Science
  • Molecules
  • Organic Materials
  • Polymers
  • Spectrometers

Fields of Study

  • Materials science

Readers

  • Nanoscale Plasmonic Nanotechnology
  • Polymer Science and Technology
  • Software Engineering

Technology Areas

  • Directed Energy