Reactions Leading to Ignition in Nanocomposite Al-oxide Systems

Abstract

Aluminum-metal oxide energetic compositions with components mixed on the nano-scale are substantially more reactive than conventional thermites and are of interest as potential additives to propellants, explosives, and pyrotechnics. For such nanocomposite materials prepared by Arrested Reactive Milling, the exothermic reactions leading to ignition were detected to begin at relatively low temperatures. These materials are prepared by mechanical processing at room temperature, and the nature of the interface present between aluminum and the oxidizer (metal oxide, e.g., CuO, MoO3, Bi2O3, etc.) is unknown. Initial estimates show that the reaction rates observed in thermo-analytical experiments cannot be explained assuming that the metal and oxidizer are separated by a substantial oxide layer, similar to that present on the surface of conventional aluminum particles. Experiments using a Thermal Activity Monitor (TAM III) quantify the reaction rates between aluminum and oxidizer at temperatures as low as 30-deg C; the results of these measurements are presented and discussed in the context of the redox reactions leading to ignition in such materials.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Mar 01, 2010
Accession Number
ADA521784

Entities

People

  • Alexandre Ermoline
  • Edward L Dreizin
  • Mirko Schoenitz

Organizations

  • Air Force Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Air Force Research Laboratories
  • Aluminum Oxides
  • Chemical Reaction Properties
  • Chemical Reactions
  • Composite Materials
  • Exothermic Reactions
  • Ignition
  • Low Temperature
  • Materials
  • Measurement
  • Metal Oxides
  • Metals
  • Nanocomposites
  • Oxidation Reduction Reactions
  • Oxide Films
  • Oxides
  • Particles

Readers

  • Combustion science or combustion engineering.
  • Nanocomposite Materials Science