Co-Generation of Acetylene and Hydrogen for a Carbide-Based Fuel System

Abstract

The co-generation of acetylene and hydrogen from the hydrolysis of calcium carbide and calcium hydride was investigated as part of a unique carbide-based fuel system intended for high-temperature fuel cells. To gain better control of this highly energetic reaction, glycerin was used to coat the reactant particles to form slurry prior to their reaction with water. This process was shown to moderate the rate of gas production, as well as to provide a means for preparing slurry that could be pumped into the reactor vessel. It was also observed that the presence of calcium hydroxide, a by-product of hydrolysis, lowered the solubility of acetylene resulting in a higher initial flow rate due to less acetylene being dissolved in solution. However, the buildup of calcium hydroxide with time inhibited the hydrolysis of both calcium carbide and calcium hydride causing the acetylene and hydrogen flow rates to decrease.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2010
Accession Number
ADA523993

Entities

People

  • A. Alan Burke
  • Lily Dubois
  • Louis G. Carreiro

Organizations

  • Naval Undersea Warfare Center

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Alkynes
  • Calcium
  • Calcium Compounds
  • Calcium Hydrides
  • Calcium Hydroxide
  • Cells
  • Chemical Synthesis
  • Chemistry
  • Energy Storage
  • Flow Rate
  • Fuel Cells
  • Fuel Systems
  • High Temperature
  • Hydrogen
  • Solid Oxide Fuel Cells
  • Storage
  • Unmanned Underwater Vehicles

Fields of Study

  • Chemistry

Readers

  • Combustion science or combustion engineering.
  • Environmental Engineering
  • Surface Engineering/Surface Coating Technology.

Technology Areas

  • Biotechnology