Final Report for contract Number W911NF-06-1-0515 (University of Florida)

Abstract

We have been investigating an electrochemical single-molecule counting experiment called nanopore resistive-pulse sensing. The sensor element is a conically shaped gold nanotube embedded in a thin polymeric membrane. We have been especially interested in counting protein molecules using these nanotube sensors. This is accomplished by placing the nanotube membrane between two electrolyte solutions, applying a transmembrane potential difference, and measuring the resulting ionic current flowing through the nanopore. In simplest terms, when a protein molecule enters and translocates the nanopore, it transiently blocks the ion current, resulting in a downward current pulse. In this way, single-molecule pore-translocation events are counted as individual current pulses. The frequency of theses current-pulse events is proportional to the concentration of the analyte, and the identity of the analyte is encoded in the current-pulse signature, as defined by the average magnitude and the duration of the current pulses. See attachment.

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Document Details

Document Type
Technical Report
Publication Date
Jul 15, 2010
Accession Number
ADA533810

Entities

People

  • C. R. Martin
  • H. Mukaibo
  • R. Crooks

Organizations

  • University of Florida

Tags

Communities of Interest

  • Advanced Electronics
  • Sensors

DTIC Thesaurus Topics

  • Abstracts
  • Agreements
  • Carbon Nanotubes
  • Contracts
  • Dacron
  • Department Of Defense
  • Detectors
  • Engineering
  • Fullerenes
  • Ionic Current
  • Mathematics
  • Membrane Potentials
  • Membranes
  • Molecules
  • Pulse Amplitude
  • Standards
  • Students

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  • Mathematics or Statistics
  • Molecular Genetics
  • Nanocomposite Materials Science