Laser Hybrid Fabrication of Nanoporous Structures on Metallic Material Surface

Abstract

This paper reports a novel approach to fabricate Cu-Mn nanoporous structures by laser deposition hybrid with electrolyte dealloying. Cu25Mn75 alloy layers free of cracks were fabricated by laser deposition onto a mild steel surface. The dendrite microstructure of the as-deposited layer was further processed by laser remelting to refine the grain size and change the morphology to be cellular crystalline. Electrolyte dealloying was then applied on the as-deposited and remelted layers. Uniform porous microstructure will form under optimized electrode current density to be about 5 mA/cm(2). The size of the porous structure decreases with the increase of laser remelting speed. Nanoporous structure is available with remelting speed up to 83 mm/s. A minimum size of nanoporous structure was achieved to be 35.2 nm up to date with this laser dealloying hybrid method. The Nanoporous Cu-Mn structure was further electrolessly plated of Ni to form a nanoporous Cu-Ni composite coating. The Cyclic voltammetry curves indicate that both the nanoporous Cu coatings and the nanoporous Cu-Ni composite coatings show electrochemical catalysis properties. The Cu-Ni composite coatings with 20 minute Ni plating demonstrates the best catalysis properties,with oxidation peak current density up to about 60 mA/cm(2).

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 2009
Accession Number
ADA540281

Entities

People

  • Changsheng Dong
  • Hongjun Zhang
  • Mingxing Ma
  • Minlin Zhong
  • Wenjin Liu
  • Yide Kan
  • Yu Gu

Organizations

  • Tsinghua University

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Advanced Materials
  • Coatings
  • Copper Coatings
  • Current Density
  • Electroless Plating
  • Fabrication
  • Grain Boundaries
  • Grain Size
  • Material Degradation Processes
  • Materials
  • Materials Processing
  • Materials Science
  • Metal Films
  • Metals
  • Porosity
  • Porous Materials
  • Porous Metals

Fields of Study

  • Materials science

Readers

  • Aerospace Engineering
  • Metallurgy
  • Surface Engineering/Surface Coating Technology.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition