Design of Energetic Ionic Liquids

Abstract

An essential need of the US Air Force is the discovery, development, and fielding of new, energetic materials for advanced chemical propulsion in space and missile applications. Some of the key factors driving the requirement for new chemical propellants include: (a) improved performance in terms of increased specific impulse and density, (b) reduced sensitivity to external stimuli such as impact, friction, shock, and electrostatic discharge, and (c) mitigation of environmental and toxicological hazards (and the resulting costs) associated with currently used propellants. A class of compounds that can potentially meet these requirements is known as ionic liquids (ILs), which are chemical salts with unusually low melting points. The physical and chemical properties of ILs render them useful for many purposes, most notably as environmentally benign (?green?) solvents/reaction media but also as catalysts, electrolytes, etc. From a Department of Defense (DoD) perspective, ILs are being explored as new propellants, explosives, and munitions. The Air Force, in particular, is interested in ILs as potential replacements for currently used monopropellants such as hydrazine?which is carcinogenic, highly toxic, and has relatively modest performance characteristics. In contrast, many ILs have superior densities and specific impulses as well as significantly reduced sensitivity and toxicity characteristics. Furthermore, their properties can be carefully tuned via the choice of the component ions. The overall objective of the Design of Energetic Ionic Liquids Challenge Project is to address several key technical issues and challenges associated with the characterization, design, and development of ILs as new monopropellants.

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Document Details

Document Type
Technical Report
Publication Date
Apr 27, 2011
Accession Number
ADA545129

Entities

People

  • Gregory A. Voth
  • Jerry A. Boatz
  • Mark S. Gordon
  • Sharon Hammes-Schiffer

Organizations

  • Air Force Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Air Force
  • Air Force Research Laboratories
  • Chemical Properties
  • Chemistry
  • Computational Science
  • Density Functional Theory
  • Department Of Defense
  • Energetic Materials
  • Ionic Liquids
  • Liquid Propellants
  • Materials
  • Military Research
  • Molecular Dynamics
  • Monopropellants
  • Phase Transformations
  • Physical Properties
  • Propellants

Readers

  • Rocket Propulsion.
  • Systems Analysis and Design

Technology Areas

  • Space
  • Space - Hall-Effect Thruster