Nanotailored Carbon Fibers

Abstract

Various spinning trials of polyacrylonitrile (PAN) and PAN/carbon nanotube (CNT) fibers were conducted using single- and bi-component spinning to obtain precursor fiber for carbonization. Materials parameters, such as homo- vs co-polymer, as well as different molecular weight polymers were investigated. In order to obtain better precursor fiber with circular cross-sectional shape, gelation bath composition and bath temperature were varied in the spinning process. The precursor fiber containing 0.5 to 1 wt% CNT exhibited tensile strength in the range of 0.6 to 1 GPa and tensile modulus in the range of 16 to 28 GPa. The PAN/CNT precursor fibers were subsequently stabilized and carbonized in the batch process by varying stabilization conditions such as tension, temperature, and residence time. The effective carbon fiber diameter from core precursor fiber was in the range of 3.5 - 4 microns. The highest average tensile strength and modulus were 5.5 GPa and 362 GPa while the maximum properties for the individual filaments were up to 6.8 GPa and 389 GPa, respectively. This study proves that PAN/CNT technology can be used to process carbon fibers with a tensile strength approaching 7 GPa and tensile modulus approaching 400 GPa at a relatively low carbonization temperature of 1300 degree C.

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Document Details

Document Type
Technical Report
Publication Date
Apr 27, 2012
Accession Number
ADA560477

Entities

People

  • Han Gi Chae

Tags

Communities of Interest

  • Advanced Electronics
  • Air Platforms

DTIC Thesaurus Topics

  • Alkenes
  • Carbon Fibers
  • Carbon Nanotubes
  • Composite Materials
  • Diameters
  • Engineered Materials
  • Fibers
  • Fullerenes
  • Materials
  • Mechanical Properties
  • Molecular Weight
  • Polymers
  • Raman Spectra
  • Tensile Modulus
  • Tensile Properties
  • Tensile Strength
  • Tensile Testing

Fields of Study

  • Materials science

Readers

  • Reinforced Composite Materials