Recombinant Reflectin-Based Optical Materials

Abstract

Reflectins are a unique group of structural proteins involved in dynamic optical systems in cephalopods that modulate incident light or bioluminescence. We describe cloning structural characterization, and optical properties of a reflectinbased domain, refCBA, from reflectin 1a of Hawaiian bobtail squid, Euprymna scolopes. Thin films created from the recombinant protein refCBA display interesting optical features when the recombinant protein is appropriately organized. RefCBA was cloned and expressed as a soluble protein enabling purification, with little structural organization found using Fourier transform infrared spectroscopy and circular dichroism. Single-layer and multi-layer thin films of refCBA were then produced by flow coating and spin coating, and displayed colors due to thin film interference. Diffraction experiments showed the assemblies were ordered enough to work as diffraction gratings to generate diffraction patterns. Nano-spheres and lamellar microstructures of refCBA samples were observed by scanning electron microscopy and atomic force microscopy. Despite the reduced complexity of the refCBA protein compared to natural reflectins, unique biomaterials with similar properties to reflectins were generated by self-assembled reflectin-based refCBA molecules.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2012
Accession Number
ADA569634

Entities

People

  • David L. Kaplan
  • Fiorenzo G Omenetto
  • Guokui Qin
  • Jason E. Bressner
  • Patrick B Dennis
  • Rajesh R Naik
  • Wendy J. Crookes-goodson
  • Xiao Hu
  • Yuji Zhang
  • Zhongyuan Sun

Organizations

  • Air Force Research Laboratory

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Amino Acids
  • Chemical Synthesis
  • Chemistry
  • Diffraction
  • Gratings (Spectra)
  • Light Sources
  • Materials
  • Materials Science
  • Microscopes
  • Microscopy
  • Optical Properties
  • Optics
  • Polymers
  • Proteins
  • Self Assembly
  • Spectra
  • Spectroscopy

Readers

  • Military History
  • Molecular Genetics
  • Thin Film Deposition Science.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene