Adsorptive Desulfurization of JP-8 Fuel Using Ag+/Silica Based Adsorbents at Room Temperature

Abstract

We report an adsorptive desulfurization of Army JP-8 fuel using silver ions (Ag+) tethered to porous silica at ambient conditions. Mesoporous silica-both one- and two-dimensional MCM-41 and MSUH, respectively-were studied as adsorbent support materials for the desulfurization of liquid phase JP-8 fuel. In this work, silver loadings up to ~33 wt.% on silica support materials were prepared and evaluated for the adsorptive desulfurization of JP-8 jet fuel. These adsorbents were characterized using JP-8 fuel containing ~400 ppmw sulfur at room temperature. The sulfur adsorption capacities of Ag+ (31.8 wt.%)/MSUH and Ag+ (32.8 wt.%)/MCM-41with static adsorption experiments were 24.0 and 26.4 mgS/g adsorbent, respectively. The sulfur adsorption capacities of Ag+ (31.8 wt.%)/MSUH, Ag+ (32.8 wt.%)/MCM-41, and Ag+ (28.1 wt.%)/ MSUH+MCM-41 with packed-bed adsorption experiments were 40.0, 31.8, and 24.3 mgS/g adsorbent, respectively. Sulfur removal and adsorption characteristics for these sorbents are described.

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Document Details

Document Type
Technical Report
Publication Date
Sep 01, 2012
Accession Number
ADA570605

Entities

People

  • Dat T. Tran
  • Deryn Chu
  • Zachary W. Dunbar

Organizations

  • United States Army Research Laboratory

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Aluminum Oxides
  • Desulfurization
  • Fuel Cells
  • Fuels
  • Jet Engine Fuels
  • Liquid Phases
  • Liquids
  • Materials
  • Measurement
  • Military Research
  • Organic Sulfur Compounds
  • Oxidation
  • Oxides
  • Particles
  • Silicon Dioxide
  • Sulfur Compounds
  • Two Dimensional

Fields of Study

  • Environmental science

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Petroleum Engineering