The Rechargeability of Silicon-Air Batteries

Abstract

This project aimed to investigate silicon-air batteries as a rechargeable power source of high energy density. Si-air batteries are an attractive possibility due to high charge capacity (approximately 4 times higher than conventional Zn-air, and nearly that of Li-air) with less safety and environmental concerns. Studies of Si-air electrochemical cells using both liquid room-temperature ionic liquid as electrolyte and a gel polymer electrolyte (formed by incorporating an ionic liquid electrolyte into polymeric matrix) were undertaken. Research challenges included overcoming the SiO2 reaction product from clogging the porous carbon-air electrode, reducing the SiO2 byproduct during recharging and redepositing the Si ions in a manner to permit continued operation without loss of energy density, and avoiding the build-up of water byproduct in the electrolyte during reduction during recharge phase. This last issue was seen as a critical roadblock for the continued development at this time, although production of H2O during operation could make an Si-air electrochemical cell a source of water for other applications.

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 2012
Accession Number
ADA570671

Entities

People

  • Yair Ein-eli

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Air Force Research Laboratories
  • Chemical Analysis
  • Chemical Synthesis
  • Chemistry
  • Dermatologic Agents
  • Electrochemical Cells
  • Electrochemical Reactions
  • Electrodes
  • Electrolytes
  • Energy
  • Ionic Liquids
  • Materials
  • Materials Engineering
  • Measurement
  • Metal Air Batteries
  • Organic Chemistry
  • Photoelectrochemical Cells

Fields of Study

  • Materials science

Readers

  • Battery Technology and Engineering
  • Polymer Science and Technology
  • Systems Analysis and Design