Superior Thermal Interface via Vertically Aligned Carbon Nanotubes Grown on Graphite Foils

Abstract

In an attempt to study the thermal transport at the interface between nanotubes and graphene, vertically aligned multiwalled carbon nanotubes (CNTs) were grown on graphite thin film substrates. A systematic cross-sectional probing of the materials morphology of the interface by scanning electron microscopy and high-resolution transmission electron microscopy revealed that an excellent bond existed between the nanotubes and the substrate along some fraction of interface. Imaging and electron diffraction analyses performed at the boundary reveal a polycrystalline interfacial structure. Compositional probing along the interface by energy dispersive x-ray spectroscopy revealed that there were no catalyst particles or other impurities present. The estimated interfacial thermal resistance of lower than 5 7.5 (mm[expn 2] K)/W suggests that this type of CNT/graphite interface could open up multiple routes toward the designing and development of advanced thermal interface materials for aerospace and nano-/microelectronics applications.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2012
Accession Number
ADA578735

Entities

People

  • Ajit K. Roy
  • Feng Du
  • Liming Dai
  • Robert W. Wheeler
  • Sabyasachi Ganguli
  • Vikas Varshney

Organizations

  • Air Force Research Laboratory

Tags

DTIC Thesaurus Topics

  • Air Force
  • Carbon Nanotubes
  • Diffraction
  • Electron Diffraction
  • Electron Microscopy
  • Films
  • Fullerenes
  • Graphene
  • Graphitic Materials
  • Materials
  • Microscopes
  • Microscopy
  • Scattering
  • Spectra
  • Thermal Conductivity
  • Thermal Diffusivity
  • Thermal Resistance

Readers

  • Materials Science and Engineering.
  • Nanocomposite Materials Science

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene
  • Space