Terahertz Science & Technology: Sensing Bio-Molecular Nanostructures & Photoinduces Transitions Between Metastable States

Abstract

Significant progress in experimental and computational sub-THz vibrational spectroscopy has been made in the last 2-3 years to improve the sensitivity of THz spectroscopic characterization of large biological molecules, microorganisms and structural elements for bio-molecular electronics. The correct choice of substrate, concentration of materials in solution or suspension, and material alignment at deposition permitted us to significantly enhance the intensities of modes in solid samples when using a Fourier transform spectrometer with a spectral resolution of 0.25/cm. The analysis of results indicates that the spectroscopic signatures of microorganisms originates from the combination of low frequency vibrational modes or group of modes at close frequencies within molecular components of bacterial cells/spores, with the significant contribution from the DNA. However, this spectral resolution still does not provide a sufficient level of discriminative capability. Highly resolved vibrational spectroscopy was demonstrated utilizing the CW frequency-domain spectroscopic sensor prototype developed by Vibratess for room temperature operation. Intense and narrow spectral resonances in transmission/absorption spectra of nano-samples from biological materials have been observed. Demonstrated multiple intense and specific signatures provide conditions for reliable discriminative capability using sub-THz frequency domain spectroscopy to the level of the strains of the same bacteria that was not possible before.

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Document Details

Document Type
Technical Report
Publication Date
Jul 31, 2012
Accession Number
ADA580384

Entities

People

  • B. Gelmont
  • I. Sizov
  • M. Lvovska
  • T. Dorofeeva
  • T. Globus
  • T. Khromova

Organizations

  • University of Virginia

Tags

Communities of Interest

  • Biomedical

DTIC Thesaurus Topics

  • Absorption Coefficients
  • Absorption Spectra
  • Bacteria
  • Biosensors
  • Chemistry
  • Detection
  • Detectors
  • Diffraction
  • Electromagnetic Fields
  • Frequency Domain
  • Macromolecules
  • Magnetic Fields
  • Measurement
  • Molecular Dynamics
  • Spectra
  • Spectral Lines
  • Terahertz Radiation

Fields of Study

  • Physics

Readers

  • Image Processing and Computer Vision.
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Microelectronics