A Highly Aromatic and Sulfonated Ionomer for High Elastic Modulus Ionic Polymer Membrane Micro-Actuators

Abstract

A high modulus, sulfonated ionomer synthesized from 4,6-bis(4-hydroxyphenyl)-N,N-diphenyl-1,3,5-triazin-2-amine and 4,40-biphenol with bis(4-fluorophenyl)sulfone (DPA-PS:BP) is investigated for ionic polymer actuators. The uniqueness of DPA-PS:BP is that it can have a high ionic liquid (IL) uptake and consequently generates a high intrinsic strain response, which is >1.1% under 1.6 V while maintaining a high elastic modulus (i.e. 600 MPa for 65 vol% IL uptake). Moreover, such a high modulus of the active ionomer, originating from the highly aromatic backbone and side-chain-free structure, allows for the fabrication of free-standing thin film micro-actuators (down to 5 m thickness) via the solution cast method and focused-ion-beam milling, which exhibits a much higher bending actuation, i.e. 43 m tip displacement and 180 kPa blocking stress for a 200 m long and 5 m thick cantilever actuator, compared with the ionic actuators based on traditional ionomers such as Nafion, which has a much lower elastic modulus (50 MPa) and actuation strain.

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Document Details

Document Type
Technical Report
Publication Date
May 01, 2012
Accession Number
ADA584103

Entities

People

  • Dean M. Tigelaar
  • Gokhan Hatipoglu
  • Mitra Yoonessi
  • Q. M. Zhang
  • Ran Zhao
  • Srinivas Tadigadapa
  • Yang Liu

Organizations

  • Virginia Tech

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies
  • Space

DTIC Thesaurus Topics

  • Actuators
  • Bulk Modulus
  • Conductivity
  • Electrical Engineering
  • Electrodes
  • Electrolytes
  • Engineering
  • Fabrication
  • Films
  • Glass Transition Temperature
  • Ionic Liquids
  • Ions
  • Materials
  • Microelectromechanical Systems
  • Modulus Of Elasticity
  • Polymer Matrix Composites
  • Transition Temperature

Readers

  • Mechanical Engineering/Mechanics of Materials.
  • Polymer Science and Technology