Controlled Hydrogen Peroxide Decomposition for a Solid Oxide Fuel Cell (SOFC) Oxidant Source with a Microreactor Model

Abstract

A microchannel reactor for hydrogen peroxide decomposition is being developed for integration with fuel cell systems that can power undersea vehicles. However, the catalytic decomposition of H2O2 is predisposed to thermal runaway. A micro-scale packed bed reactor (MPBR), theoretically capable of inhibiting thermal runaway, is under development in COMSOL to illustrate thermal management and oxygen production during this reaction. The COMSOL model solves mass, energy, and momentum balances to simulate temperature and concentration profiles within the reactor. Using a stainless steel block around the capillary to act as an extended surface for higher heat removal rates and an initial volumetric flow rate of 2e(-9) m(3)/s \201about 0.1 ml/min), a temperature rise less than 8 K was simulated and an outlet concentration of 1716 mol/m(3) oxygen was achieved. Overall the results indicate that thermally-controlled oxygen generation from hydrogen peroxide decomposition is feasible in a microreactor provided there is sufficient external surface area to facilitate convective cooling.

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Document Details

Document Type
Technical Report
Publication Date
Oct 01, 2007
Accession Number
ADA591387

Entities

People

  • A. Burke
  • E. Lennon
  • R. Besser

Organizations

  • Stevens Institute of Technology

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Cells
  • Chemical Reactions
  • Energy
  • Flow Rate
  • Fluids
  • Fuel Cells
  • Heat Energy
  • Heat Of Activation
  • Heat Transfer
  • Latent Heat
  • Navier Stokes Equations
  • Rocket Oxidizers
  • Solid Oxide Fuel Cells
  • Stainless Steel
  • Temperature Control
  • Three Dimensional
  • Unmanned Underwater Vehicles

Readers

  • Combustion and Flow Dynamics.
  • Combustion science or combustion engineering.
  • Electrochemical Engineering/ Fuel Cell Technologies

Technology Areas

  • Biotechnology