Glycopeptides as Analgesics: Non-Toxic Alternatives to Morphine for Combat Casualty Care

Abstract

Background: Endogenous opiate peptides (enkephalins and endorphins) are more potent and specific than morphine and congeners. Specificity is determined by the "address segment" while binding is determined by the "message segment." Incorporation of carbohydrates into the address segment results in improved biodistribution and enhanced penetration of the blood-brain barrier (BBB). Thus, glycosylation of mu- or delta-selective peptides allows the resulting glycopeptides to be used as potent and safer alternatives to classical opiates such as morphine. Morphine and other muselective agonists are immunosuppressants, while the glycopeptide enkephalins are selective delta-agonists, which are known to be immunostimulants. Hypothesis: Enkephalin transport and penetration of the blood-brain barrier can be determined by reversible binding to membranes, which may be manipulated by altering the amphipathicity of the address segment directly by introduction of hydrophilic sugar moieties, and lipophilic side chains. Conclusion: Glycopeptide analogues of enkephalins are viable drug candidates. Obstacles regarding the synthesis and design of analgesics have been overcome. Further studies are required in order to meet FDA requirements. See attached .pdf file (14 pg and 22 pg reviews) for details.

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Document Details

Document Type
Technical Report
Publication Date
Dec 05, 2013
Accession Number
ADA594872

Entities

People

  • Robin Polt

Organizations

  • University of Arizona

Tags

DTIC Thesaurus Topics

  • Chemical Synthesis
  • Chemistry
  • Drug Abuse
  • Health Services
  • Medical Personnel
  • Membrane Lipids
  • Military Hospitals
  • Organic Chemistry
  • Peptides
  • Pharmacology
  • Rodents
  • Therapy

Fields of Study

  • Biology
  • Chemistry

Readers

  • Immunology
  • Molecular and Cellular Biochemistry
  • Neurotrauma and Rehabilitation Medicine.