Crossover from Incoherent to Coherent Phonon Scattering in Epitaxial Oxide Superlattices
Abstract
Elementary particles such as electrons or photons are frequent subjects of wave-nature-driven investigations, unlike collective excitations such as phonons. The demonstration of wave particle crossover, in terms of macroscopic properties, is crucial to the understanding and application of the wave behaviour of matter. We present an unambiguous demon- stration of the theoretically predicted crossover from diffuse (particle-like) to specular (wavelike) phonon scattering in epitaxial oxide superlattices, manifested by a minimum in lattice thermal conductivity as a function of interface density. We do so by synthesizing superlattices of electrically insulating perovskite oxides and systematically varying the interface density, with unit-cell precision, using two different epitaxial- growth techniques. These observations open up opportuni- ties for studies on the wave nature of phonons, particularly phonon interference effects, using oxide superlattices as model systems, with extensive applications in thermoelectrics and thermal management.
Document Details
- Document Type
- Technical Report
- Publication Date
- Dec 08, 2013
- Accession Number
- ADA605255
Entities
People
- Ajay K Yadav
- Arsen Soukiassian
- Brian M. Foley
- Che-hui Lee
- Jayakanth Ravichandran
- John C. Duda
- Pim B. Rossen
- Ramez Cheaito
- S. J. Suresha
- Ye Zhu
Organizations
- University of Virginia