Continuous Ultra-Thin MOS2 Films Grown by Low-Temperature Physical Vapor Deposition (Postprint)

Abstract

Uniform growth of pristine two dimensional (2D) materials over large areas at lower temperatures without sacrifice of their unique physical properties is a critical pre-requisite for seamless integration of next-generation van der Waals heterostructures into functional devices. This Letter describes a vapor phase growth technique for precisely controlled synthesis of continuous, uniform molecular layers of MoS2 on silicon dioxide and highly oriented pyrolitic graphite substrates of over several square centimeters at 350 deg C. Synthesis of few-layer MoS2 in this ultra-high vacuum physical vapor deposition process yields materials with key optical and electronic properties identical to exfoliated layers. The films are composed of nano-scale domains with strong chemical binding between domain boundaries, allowing lift-off from the substrate and electronic transport measurements from contacts with separation on the order of centimeters.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 2014
Accession Number
ADA608958

Entities

People

  • Andrey A. Voevodin
  • Benjamin Wang
  • Christopher Muratore
  • J. E. Bultman
  • Jianjun Hu
  • M. L. Jespersen
  • Michael E. McConney
  • Mohammad Ariful Haque
  • P. J. Shamberger
  • R. D. Naguy

Organizations

  • Air Force Research Laboratory

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Air Force
  • Air Force Research Laboratories
  • Crystal Lattices
  • Energy
  • Films
  • Graphitic Materials
  • High Vacuum
  • Low Temperature
  • Materials
  • Materials Engineering
  • Materials Processing
  • Measurement
  • Molecular Orbital Theory
  • Physical Properties
  • Physical Vapor Deposition
  • Two Dimensional
  • Vapor Deposition

Fields of Study

  • Physics

Readers

  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.
  • Thin Film Deposition Science.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene