Layer-by-Layer Assembly of Halogen-Free Polymeric Materials on Nylon/Cotton Blend for Flame Retardant Applications

Abstract

Thin films of environmentally safe, halogen free, anionic sodium phosphate and cationic polysiloxanes were deposited on a Nyco (1:1 nylon/cotton blend) fabric via layer-by-layer (LbL) assembly to reduce the inherent flammability of Nyco fabric. In the coating process, we used three different polysiloxane materials containing different amine groups including 35-45% (trimethylammoniummethylphenythyl)-methyl siloxane-55-65% dimethyl siloxane copolymer chloride salt (QMS-435), aminoethylaminopropyl silsesquioxane-methylsilsesquioxane copolymer oligomer (WSA-7021) and aminopropyl silesquioxane oligomers (WSA-991) as a positive polyelectrolyte. Thermo-gravimetric analysis showed that coated fabric has a char yield around 40% at 600 degrees C whereas control fabric is completely consumed. The vertical flame test (VFT) on the LbL-coated Nyco fabric was passed after a flame time of 2 s, with a char length of 3.81 cm. Volatile and nontoxic degradation products of flame retardant-coated fabric were analyzed by pyrolysis gas chromatography mass spectroscopy (Py-GCMS). Surface morphology of coated fabrics and burned fabric residues were studied by scanning electron microscopy.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Jul 01, 2015
Accession Number
ADA622125

Entities

People

  • Jayant Kumar
  • Mahesh Narkhede
  • Ravi Mosurkal
  • Sammaiah Thota
  • Wayne S. Muller

Organizations

  • University of Massachusetts Lowell

Tags

Communities of Interest

  • Advanced Electronics
  • Biomedical
  • Cyber

DTIC Thesaurus Topics

  • Alkenes
  • Biomedical And Dental Materials
  • Cellulose
  • Chemical Synthesis
  • Chemistry
  • Films
  • Flame Retardants
  • Gas Chromatography
  • Mass Spectroscopy
  • Materials
  • Materials Science
  • Microscopy
  • Organic Chemistry
  • Polymer Degradation
  • Polymers
  • Spectroscopy
  • Thin Films

Fields of Study

  • Materials science

Readers

  • Manufacturing Engineering.
  • Polymer Science and Engineering.
  • Polymer Science and Technology

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene