Exciton-dominant Electroluminescence from a Diode of Monolayer MoS2

Abstract

In two-dimensional monolayer MoS2, excitons dominate the absorption and emission properties. However, the low electroluminescent efficiency and signal-to-noise ratio limit our understanding of the excitonic behavior of electroluminescence. Here, we study the microscopic origin of the electroluminescence from a diode of monolayer MoS2 fabricated on a heavily p-type doped silicon substrate. Direct and bound-exciton related recombination processes are identified from the electroluminescence. At a high electron-hole pair injection rate, Auger recombination of the exciton-exciton annihilation of the bound exciton emission is observed at room temperature. Moreover, the efficient electrical injection demonstrated here allows for the observation of a higher energy exciton peak of 2.255 eV in the monolayer MoS2 diode, attributed to the excited exciton state of a direct-exciton transition.

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Document Details

Document Type
Technical Report
Publication Date
May 14, 2014
Accession Number
ADA624401

Entities

People

  • Hanyu Zhu
  • Majid Gharghi
  • Mervin Zhao
  • Xiang Zhang
  • Xiaobo Yin
  • Ye Yu
  • Yuan Wang
  • Ziliang Ye

Organizations

  • University of California, Berkeley

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies
  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Absorption
  • Air Force
  • Band Gaps
  • Band Structures
  • Carbon Nanotubes
  • Electroluminescence
  • Electron Holes
  • Electrons
  • Emission
  • Energy Bands
  • Excitons
  • High Energy
  • Low Temperature
  • Monomolecular Films
  • Spectra
  • Transitions
  • Two Dimensional

Readers

  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.
  • Semiconductor Device Technology

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene