A New Paradigm to Identify Reaction Pathways in Gas-phase

Abstract

The complexity of the energy landscapes of hydrocarbon molecules during combustion processes, often composed by several hundreds of minima and even more barriers, makes the heuristic search of the most likely reactions an unfeasible task even with today's computer power. As a consequence, the main advancements in the field of combustion chemistry and kinetic mechanisms development are based on "chemical intuition" and trial and error procedures, which are error prone and hard to automate. In this proposal we present a new paradigm to determine reaction pathways for gas-phase species that relies on two major components: molecular dynamics simulations and advanced sampling techniques. Molecular dynamics (MD) in conjunction with advanced sampling techniques, such as Metadynamics, are used to explore the energy landscapes of uni-molecular and bi-molecular reactions in gas phase. Starting from the fuel molecule and running several simulations from the various wells identified withMD, we can recover a network of reactions that includes a controlled number of reactions, allowing the construction of reaction pathways with the desired level of detail.

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Document Details

Document Type
Technical Report
Publication Date
Apr 27, 2015
Accession Number
ADA625499

Entities

People

  • Angela Violi
  • Paolo Elvati

Organizations

  • University of Michigan

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Air Force Research Laboratories
  • Algorithms
  • Chemical Reactions
  • Combustion
  • Computational Chemistry Methods
  • Decomposition
  • Dynamics
  • Electronic Mail
  • Energy
  • Energy Transfer
  • Equations
  • Molecular Dynamics
  • Molecules
  • Potential Energy
  • Probability
  • Simulations
  • Two Dimensional

Readers

  • Combustion science or combustion engineering.
  • Distributed Systems and Data Platform Development
  • Groundwater Contamination Remediation.