Understanding the Scientific Basis of Electrocaloric Effect in Defects Modified Ferroelectric Polymers

Abstract

Materials with large electrocaloric effect (ECE) is attractive for Army and DoD applications such as for the thermal management of soldier s in battle field, cooling of electronic systems, and mobile cooling units with high cooling power, compact size, and high efficiency. Recent experiments have demonstrated large ECE in the relaxor ferroelectrics (defects modified ferroelectrics) over broad temperatures. Ferroelectrics provide a strong coupling of polarization to the applied field (easy to induce a large polarization) and the defects structures can be employed to the ployed to facially tailor the randomness of dipoles to achieve large ECE. This program develops fundamental understanding of large ECE in the relaxor ferroelectrics.Through experimental study and thermodynamics analysis, we intend to address these questions: (a) what are the polarization responses in these complex and highly coupled polar-materials that control the entropy change in the materials and (b) how to influence these polarization responses and consequently ECE via various molecular and nanocomposite approaches.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Dec 19, 2014
Accession Number
ADA626281

Entities

People

  • Lei Zhu
  • Qiming Zhang

Organizations

  • Pennsylvania State University

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Ceramic Materials
  • Chemistry
  • Composite Materials
  • Copolymers
  • Dielectric Properties
  • Dielectrics
  • Materials Processing
  • Materials Science
  • Nanocomposites
  • Nanoparticles
  • Phase Diagrams
  • Phase Transformations
  • Specific Heat
  • Thick Films
  • Thin Films
  • Transition Temperature
  • Two Dimensional

Readers

  • Materials Science and Engineering.
  • Systems Analysis and Design
  • Thermal Physics or Thermal Science.

Technology Areas

  • Microelectronics