Temperature Dependences for the Reactions of Ar+, O2+, and C7H7+ with Toluene and Ethylbenzene

Abstract

We have studied the reactions of Ar+, O-2(+), and C2H2* with toluene (CH3-C6H5) and ethylbenzene (C2H5-C6H5) as a function of temperature. Ar+ reacts with C7H8 at the collision rate constant at both 300 and 500 K to produce mainly C7H7+ cations (similar to 85%), with the remainder of the reactivity divided into numerous small channels. The fraction of C7H7+ produced as benzylium(+) (6 membered ring, Bz(+)) as opposed to tropylium(+) (7 membered ring, Tr+) is determined through ion-molecule reactivity to be primarily Bz(+). The reaction of Ar+ with C8H10 proceeds at slightly lower than the collision rate constant at 300 K, but increases to the collision rate constant at 500 K. Over 80% of the products were C7H7+, the large majority of which also is Bz(+). The O-2(+) reaction with C8H10 proceeds at the collision rate constant and produces C8H10+, C6H6+, and C7H7+, with the latter again primarily being Bz(+). C7H7+ was found to react with both CH3-C6H5 and C2H5-C6H5 by both collisionally stabilized clustering and a bimolecular reaction forming R-C6H4-CH2+. At 300 K the rate constants are about half of the collision rate constant and drop rapidly with temperature. About 2/3 of the products are clusters at 300 K, 1/3 at 400 K, and negligible amounts at 500 and 600 K. Evidence for thermal dissociation of the cluster is presented. Calculations show the most stable structure is the one where the methylene group of benzylium is coordinated at the para position of the alkylbenzene, with one phenyl group approximately 45 degrees out of plane relative to the other. A bond strength of 15-16 kcal mol(-1) is calculated for both neutrals. Numerous less stable structures were found.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Jul 01, 2013
Accession Number
ADA626630

Entities

People

  • Albert A Viggiano
  • Joshua J Melko
  • Nicholas S Shuman
  • Shaun G Ard

Organizations

  • Air Force Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies
  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Air Force
  • Air Force Research Laboratories
  • Charge Transfer
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemistry
  • Clustering
  • Collisions
  • Dissociation
  • Electrons
  • Ionization
  • Mass Spectrometry
  • Measurement
  • Molecules
  • Physical Chemistry
  • Reactivities
  • Spacecraft

Fields of Study

  • Chemistry

Readers

  • Molecular Photonics/Laser Physics
  • Organic Chemistry