The Viscoelastic Properties of Crosslinked Poly(Ethylene Tetrasulfide) Polymers.

Abstract

A range of crosslink densities have been introduced into poly(ethyl tetrasulfide) by use of the trifunctional agent, 1,2,3-tricholoropropane. The formation of a crosslinked structure has been established by torsional modulus measurements over a range of temperatures from the glass transition region to a region of rapid stress decay due to interchange reactions between polysulfide linkages. Estimates have been made of the deviation from ideal rubber elasticity by calculating the front factors. The density of crosslinked poly(ethyl acrylate) was found to increase with the amount of crosslinking up to 35% crosslinking agent, and then to fall steeply at higher crosslink densities. Samples containing less than 5% crosslinking agent showed evidence of crystallization. (Author-PL).

Document Details

Document Type
Technical Report
Publication Date
Apr 19, 1962
Accession Number
ADA952750

Entities

People

  • Arthur V. Tobolsky
  • G. D. T. Owen
  • R. B. Beevers

Organizations

  • Princeton University

Tags

DTIC Thesaurus Topics

  • Acrylates
  • Acyclic Hydrocarbons
  • Alkenes
  • Chemical Compounds
  • Crystallization
  • Elastic Properties
  • Ethylenes
  • Hydrocarbons
  • Measurement
  • Organic Compounds
  • Transition Temperature
  • Transitions

Fields of Study

  • Materials science

Readers

  • Mathematics or Statistics
  • Polymer Science and Technology