Al2O3.H2O-SiO2 Sol-Gel HR-Coatings for High-Power Laser Applications,

Abstract

Pursuing our official collaborative ICF-laser search and development program at Limeil National Laboratory (LNL) with the Lawrence Livermore National Laboratory (LLNL) for high damage threshold optical coatings, we have now formally established that Sol-Gel highly reflective coatings prepared from colloids are superior to those prepared from solutions of precursor materials. Thus, single layer coatings of bohemite A12 O3.H2 0 have been prepared on fused silica and BK-7 substrates from aqueous colloidal suspensions of hydrated alumina at room temperature . Such coatings were porous and therefore revealed a measured refractive index of about 1.44, lower than the relevant dense material. These single coats when laser damage tested, have exhibited thresholds, under S-on-1 irradiation mode (S shots at the same fluence onto a selected site) of respectively 12-14 J/cm2 with 3-ns pulses and 35-50 J/cm2 with-16 ns pulses at 30-Hz. Multilayer, high reflectivity, dielectric coatings were also prepared at room temperature by laying down quarterwave-thick, alternating coats of this alumina with silica also prepared from colloidal sol, and having a refractive index of 1.22. To achieve 99 % reflectivity 32 to 36 total layers were required. Such HR-coatings revealed damage thresholds as good as those of single layers of the constituting oxides in the same laser conditions.

Document Details

Document Type
Technical Report
Publication Date
Mar 01, 1992
Accession Number
ADP006435

Entities

People

  • H. G. Floch
  • J. J. Priotton

Organizations

  • Lawrence Livermore National Laboratory

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Advanced Materials
  • Coatings
  • Damage
  • Engineered Materials
  • Laser Applications
  • Laser Damage
  • Lasers
  • Materials
  • Materials Laboratories
  • Optical Coatings
  • Optical Materials
  • Optics
  • Plasmonic Materials
  • Reflectivity
  • Refractive Index
  • Substrates

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Optical Physics and Photonics.
  • Pulsed Power and Plasma Physics.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition