Sol-Gel Processing of Lithium Niobate Thin-Layers for Optical Applications,

Abstract

The sol-gel processing of lithium niobate thin-layers on silicon from heterometallic alkoxide solutions is described. Advantages of sol-gel processing for low-temperature formation of stoichiometric lithium niobate are discussed. A recyrstallization procedure, involving a bimetallic alkoxide, was developed for the purification of alkoxide solutions. The alkoxide complex contained the appropriate cation ratio for the preparation of stoichiometric lithium niobate. Solvent selection, addition of nitric acid or ammonium hydroxide, and thermal processing conditions were shown to affect the ceramic microstructures. In particular, the solvent system and additives influenced grain growth and porosity in the crystallized layers. Methoxyethanol-derived layers had a grain size approximately twice that observed for the ethanol system. Use of a rapid heating process produced dense layers at 650 degC, whereas oxygen treatments allowed for crystallization at 400 degC

Document Details

Document Type
Technical Report
Publication Date
Mar 01, 1992
Accession Number
ADP006448

Entities

People

  • David A. Payne
  • Dennis J. Eichorst

Organizations

  • University of Illinois Urbana–Champaign

Tags

Communities of Interest

  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Grain Growth
  • Grain Size
  • Hydroxides
  • Lithium
  • Lithium Niobates
  • Low Temperature
  • Niobates
  • Nitric Acid
  • Piezoceramics
  • Transition Temperature

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Organic Chemistry
  • Thin Film Deposition Science.