Device Effects of Various Zr/Ti Ratios of PZT Thin-Films Prepared by SOL-GEL Method,

Abstract

PZT, PbZr sub x Tl sub 1-x 03, thin-films with various Zr/Ti ratios, 1 00/0 (lead zirconate) to 0/100 (lead titanate), were prepared by the sol-gel method. Basic electric properties, dielectric constant, tan sigma, P-E hysteresis curve, switching properties were measured respectively as a function of composition. Dielectric constant indicated a specific peak value (approximately 1100) around the morphotropic phase boundary between tetragonal and rhombohedral phase. Satisfactory low-voltage saturated hysteresis curves were observed for the compositions of PZT(90/10) through PZT(20/80). The remanent polarization and the coercive field increased as the titanium content decreased. The result of X-ray measurement showed that the lattice constants of thin-Film PZT are different from bulk ceramics for compatible compositions. The boundary, on which the c/a ratio must be 1 (rhombohedral phase), was slightly shifted to PbTiO3 side. This distortion in crystal structure is considered to be due to the thin-film effect, which the lattice mismatch between the platinum substrate and the PZT layer, restricted the ions to position into proper cites.

Document Details

Document Type
Technical Report
Publication Date
Apr 05, 1991
Accession Number
ADP006648

Entities

People

  • C. A. Paz De Araujo
  • Hideo Watanabe
  • T. Mihara

Organizations

  • University of Colorado, at Colorado Springs

Tags

DTIC Thesaurus Topics

  • Boundaries
  • Colorado
  • Crystal Structure
  • Crystals
  • Dielectric Permittivity
  • Films
  • Hysteresis
  • Lead Titanates
  • Low Voltage
  • Peak Values
  • Piezoelectric Crystals
  • Thin Films
  • Titanates
  • Titanium
  • X Rays

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.