Nanoscale Decoration of Electrode Surfaces with an STM

Abstract

The tip of a scanning tunneling microscope (STM) has been used to deposit nanometer-sized clusters of copper or silver on bare and thiol-covered gold electrode surfaces at predetermined positions. First, metal is deposited electrochemically onto the STM tip, then the clusters are formed by a jump-to-contact between the tip and the substrate during a short and very controlled approach of the tip towards the surface. When Ni is deposited Onto the tip, the jump-to-contact occurs in the opposite direction leaving holes in the gold surface. The stability of the metal clusters against anodic dissolution is discussed. Finally, it is shown how the tip approach can be used to determine tunnel barriers at the metal-electrolyte interface.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
May 30, 1999
Accession Number
ADP011200

Entities

People

  • D. M. Kolb
  • G. E. Engelmann
  • J. C. Ziegler

Organizations

  • Ulm University

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Aqueous Solutions
  • Chemical Properties
  • Electrodes
  • Electrolytes
  • Electronic Mail
  • Fabrication
  • Films
  • High Voltage
  • Low Temperature
  • Materials
  • Materials Processing
  • Monomolecular Films
  • Self Assembled Monolayers
  • Substrates
  • Technical Information Centers
  • Tunnels
  • Voltage

Fields of Study

  • Physics

Readers

  • Electrical Engineering
  • Electrochemical Engineering/ Fuel Cell Technologies
  • Materials Science and Engineering.