Physical Properties of Doped Chalcogenide Glassy Semiconductors Which are Governed by the Interaction of Negative-U Defects and Impurity States
Abstract
According to the paper the appearance of clusters with z>z(0) very important for effective doping process. It is known that CGS have soft, labile atomic structure with a great number lone-pair (LP) electrons of chalcogenide atoms, which do not take part in a net of CGS covalent bonds. These facts together with a disorder provide a fulfillment of famous 8-N rule and inefficiency of CGS doping. More rigid atomic structure of clusters prevents a fulfillment of 8-N rule and allows to exist donor- and acceptor-like electronic impurity states inside the clusters. Then "official" doping elements (Bi and Ni in our cases) together with CGS atoms (As and Se) play role of the main constituent atoms of clusters. Therefore the real chemical nature of donor or acceptor like electronic impurity states must be determined in each individual case and may not coincides with the "official" doping elements.
Document Details
- Document Type
- Technical Report
- Publication Date
- Jun 01, 2001
- Accession Number
- ADP011505
Entities
People
- K. D. Tsendin
Organizations
- Russian Academy of Sciences