Calculations of Third-Order Electronic Susceptibility of Alkali Halides
Abstract
Hyper-Raman scattering by the zone-centre optical phonons in some alkali halides is investigated. In our calculations we relate the electrooptic part of the hyper-Raman tensor to the third-order optical susceptibility and the electric field associated with the LO phonons. The results obtained for those alkali halides for which the third-order optical susceptibility has not been measured yet, show that the electrooptic and lattice contributions to the hyper-Raman scattering are comparable. In all crystals considered, we found the cubic anisotropy of the electrooptic part of the hyper-Raman tensor to be not strongly exhibited.
Document Details
- Document Type
- Technical Report
- Publication Date
- Jan 01, 2001
- Accession Number
- ADP011892
Entities
People
- Fray De Landa Castillo-alvorado
- Piotr J. Górski
- Rafal Ledzion
- Wlodzimierz Kucharczyk