Thermal Fixing of Holographic Gratings in Nearly Stoichiometric LiNbO3 Crystals
Abstract
The thermal decay of holographic gratings recorded using the conventional two-wave mixing technique has been studied in congruent and nearly stoichiometric LiNbO3 crystals doped with Mn. The activation energies of this process have been determined in the 70-130 deg C range for congruent and 20-80 deg C range for nearly stoichiometric crystals, the obtained values being 1.06 +/- 0.03 and 1.10 +/- 0.03 eV, respectively. The kinetics of the OH(-) absorption spectrum has also been studied in undoped nearly stoichiometric LiNbO3 between 40-120 deg C. The time dependence of the band intensities can be characterized by exponential time constants obeying the Arrhenius-law. The average activation energy, E(sub a) approx. 1.1 +/- 0.1 eV is in good agreement with those obtained from the thermal decay indicating that the hologram fixing process in nearly stoichiometric LiNbO3 is governed by proton migration.
Document Details
- Document Type
- Technical Report
- Publication Date
- Jan 01, 2001
- Accession Number
- ADP011902
Entities
People
- Gabor Mandula
- Krisztian Lengyel
- Laszlo Kovacs
- Mostafa A. Ellabban
- Romano A. Rupp
Organizations
- Hungarian Academy of Sciences