Stokes and Anti Stokes Luminescence in LiTaO3:Ho

Abstract

The paper deals with the excitation and decay of excited states of holmium in LiTaO3 single crystals. Particular attention is paid to processes governing a population build up on the (sup 5 S sub 2) and (sup 5 I sub 7) metastable states whose quantum efficiencies are sufficiently high to be considered as initial levels for a laser transition. We observed for the first time, to our knowledge, an efficient conversion of the 647.1 nm light of a krypton ion laser into green luminescence in the material studied. Based upon analysis of excited state relaxation dynamics it is concluded that the mechanism involved is the excited state absorption from the long lived (sup 5 I sub 7) level. Efficient single wavelength excitation is due to coincidence of transition energies of the ground state absorption and excited state absorption.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2001
Accession Number
ADP011933

Entities

People

  • G. Dominiak-dzik
  • I. Sokolska
  • P. Solarz
  • S. Golab
  • W. Ryba-romanowski

Organizations

  • Polish Academy of Sciences

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Argon Lasers
  • Crystals
  • Electronic Materials
  • Energy
  • Energy Levels
  • Energy Transfer
  • Excitation
  • Experimental Data
  • Ion Lasers
  • Lasers
  • Luminescence
  • Materials
  • Single Crystals
  • Spectra
  • Transitions

Fields of Study

  • Physics

Readers

  • Optical Physics and Photonics.
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.
  • Spectroscopy.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Quantum Computing