Optical Properties of Li2B4O7 Glasses Doped with Rare-Earths and Transition Metal Ions

Abstract

Absorption and emission spectra of Cr, Eu and Dy ions in Li2B4O7 glasses melted in oxygen and hydrogen were measured for valency states and excited states analysis. It was stated that the presence of Cr(6+) ion is limited by composition of the starting mixture and atmosphere of the melting and that this ion arises as Cr(6+)O4 complex. The 308 nm line excites the Li2B4O7:Cr glass within the highest absorption peak which can be ascribed to the following charge transfer transition: Cr(6+)O4(3d(sup 0)2p(sup 6)) right arrow Cr(5+)O(-)(3d(sup 1)2p(sup 5)). Under gamma irradiation Cr(6+)O4 complex of 3d(sup 0) configuration can be disintegrated giving additional absorption bands of Cr(3+) and may be Cr(4+) centers at tetrahedral sites One of these additional absorption bands is responsible for 430 nm emission.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2001
Accession Number
ADP011934

Entities

People

  • A. Majchrowski
  • Cz. Koepke
  • K. Wisniewski
  • M. Grinberg
  • S. M. Kaczmarek

Organizations

  • Military University of Technology

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Atmospheres
  • Charge Transfer
  • Crystals
  • Emission
  • Emission Spectra
  • Ground State
  • Hydrogen
  • Luminescence
  • Materials
  • Measurement
  • Optical Properties
  • Spectra
  • Surface Acoustic Waves
  • Transition Metals
  • Transitions

Readers

  • Materials Science and Engineering.
  • Molecular Photonics/Laser Physics
  • Spectroscopy.