Observation of the Verwey Transition in Fe3O4 Nanocrystals

Abstract

The electronic properties of arrays and isolated magnetite nanocrystals were studied using tunneling spectroscopy. Macroscopic tunnel junctions were used to study stacked arrays of the nanocrystals. The temperature dependent resistance measurements showed an abrupt increase of the resistance around 100 K, attributed to the Verwey metal-insulator transition, while the current-voltage characteristics exhibit a sharp transition from an insulator gap to a peak in the density of states near the Fermi energy. This conductance peak was sensitive to in-plane magnetic field showing large magnetoresistance. The tunneling spectra obtained on isolated particles using a Scanning Tunneling Microscope exhibit a gap-like structure below the transition temperature that gradually disappeared with increasing temperature, ending with a small peak structure around zero bias.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2003
Accession Number
ADP014326

Entities

People

  • Amos Sharoni
  • David Katz
  • Gil Markovich
  • Pankaj Poddar
  • Tcipi Fried

Organizations

  • Hebrew University of Jerusalem

Tags

Communities of Interest

  • Air Platforms

DTIC Thesaurus Topics

  • Chemistry
  • Electron Microscopy
  • Electrons
  • Fermi Levels
  • Magnetic Fields
  • Magnetoresistance
  • Materials
  • Materials Science
  • Nanocrystals
  • Nanomaterials
  • Nanotechnology
  • Observation
  • Particles
  • Phase Transformations
  • Resistance
  • Transition Temperature
  • Transitions

Fields of Study

  • Physics

Readers

  • Mathematics or Statistics
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene