Multiscale Simulation of Chemically Reactive Materials

Abstract

Project Abstract This project involves the development and application of accurate coarse-grained (CG) representations of condensed phase systems. The research effort will be devoted to greatly extending the range of rigorous coarse-graining methodology to include the possibility of chemical reactivity given that such reactive CG methods do not presently exist. The chemical reactivity will be included in both an implicit and explicit fashion. The project will also develop a new computational method called “Quantum Mechanics/Coarse-grained Mechanics” (QM/CGM) which is similar in spirit to the well known QM/MM method, but the QM in this new method is directly embedded into a CG environment. This approach will greatly accelerate QM data generation since fewer environmental motions need to be sampled since such sampling requires an expensive QM calculation. The combined set of new computational methods will also be applied to understand and potentially help design more stable electrolytes and dielectrics for energy conversion and storage problems of relevance to the Navy

Document Details

Document Type
DoD Grant Award
Publication Date
Aug 12, 2016
Source ID
N000141512493

Entities

People

  • Gregory A. Voth

Organizations

  • Office of Naval Research
  • United States Navy
  • University of Chicago

Tags

Readers

  • Computational Fluid Dynamics (CFD)
  • Quantum Chemistry

Technology Areas

  • Quantum Computing